Jpn. J. Appl. Phys. 45 (2006) pp. L450-L452  |Previous Article| |Next Article|  |Table of Contents|
|Full Text PDF (145K)| |Buy This Article|

Letter

Photoluminescence from Si Nanocrystals Embedded in In Doped SiO2

Kimihisa Matsumoto1, Minoru Fujii2 and Shinji Hayashi1, 2

1Graduate School of Science and Technology, Kobe University, Rokkodai, Nada-ku, Kobe 657-8501, Japan
2Department of Electrical and Electronics Engineering, Faculty of Engineering, Kobe University, Rokkodai, Nada-ku, Kobe 657-8501, Japan

(Received March 2, 2006; accepted March 15, 2006; published online April 14, 2006)

The luminescence properties of Si nanocrystals grown in In doped SiO2 thin films are studied. It is shown that the luminescence properties depend strongly on the In concentration. At the In concentration of smaller than 0.46 at. %, the photoluminescence (PL) intensity increases with increasing the In concentration, while the PL lifetime is nearly independent of the In concentration. This result indicates that the number of Si nanocrystals contributing to PL increases by In doping. When the In concentration exceeds 0.46 at. %, the PL intensity starts to decrease. The quenching is accompanied by the shortening of the lifetime, suggesting that nonradiative processes are introduced by In doping. However, even at a relatively high In concentration (∼3 at. %), the PL intensity is larger than that of Si nanocrystals in pure SiO2.

URL: http://jjap.jsap.jp/link?JJAP/45/L450/
DOI: 10.1143/JJAP.45.L450


|Full Text PDF (145K)| |Buy This Article| Citation:


References | Citing Articles (3)

  1. L. T. Canham: Appl. Phys. Lett. 57 (1990) 1046[AIP Scitation].
  2. M. V. Wolkin, J. Jorne, P. M. Fauchet, G. Allan and C. Delerue: Phys. Rev. Lett. 82 (1999) 197[APS].
  3. L. E. Brus: in Semiconductor and Semimetals, ed. D. J. Lockwood (Academic, New York, 1998) Vol. 49, p. 303.
  4. G. Allan, C. Delerue and M. Lannoo: Phys. Rev. Lett. 76 (1996) 2961[APS].
  5. H. Takagi, H. Ogawa, Y. Yamamoto, A. Ishizaki and T. Nakagiri: Appl. Phys. Lett. 56 (1990) 2379[AIP Scitation].
  6. S. Schuppler, S. L. Friedman, M. A. Marcus, D. L. Adler, Y.-H. Xie, F. M. Ross, Y. J. Chabal, T. D. Harris, L. E. Brus, E. E. Chaban, P. F. Szajowski, S. B. Christman and P. H. Citrin: Phys. Rev. B 52 (1995) 4910[APS].
  7. Y. Kanemitsu: in Semiconductor and Semimetals, ed. D. J. Lockwood (Academic, New York, 1998) Vol. 49, p. 157.
  8. Y. Kanemitsu, T. Futagi, T. Matsumoto and H. Mimura: Phys. Rev. B 49 (1994) 14732[APS].
  9. K. Matsumoto, M. Inada, I. Umezu and A. Sugimura: Jpn. J. Appl. Phys. 44 (2005) 8742[JSAP].
  10. K. Sato, T. Izumi, M. Iwase, Y. Show, H. Morisaki, T. Yaguchi and T. Kamino: Appl. Surf. Sci. 216 (2003) 376[CrossRef].
  11. D. Kovalev, H. Heckler, G. Polisski and F. Koch: Phys. Status Solidi B 215 (1999) 871[CrossRef].
  12. G. Polisski, H. Heckler, D. Kovalev, M. Schwartzkopff and E. Koch: Appl. Phys. Lett. 73 (1998) 1107[AIP Scitation].
  13. S. Takeoka, M. Fujii, S. Hayashi and K. Yamamoto: Phys. Rev. B 58 (1998) 7921[APS].
  14. S. Takeoka, M. Fujii and S. Hayashi: Phys. Rev. B 62 (2000) 16820[APS].
  15. W. L. Wilson, P. F. Szajowski and L. E. Brus: Science 262 (1993) 1242[Science].
  16. A. L. Efros, M. Rosen, B. Averboukh, D. Kovalev, M. Ben-Chorin and F. Koch: Phys. Rev. B 56 (1997) 3875[APS].
  17. M. Fujii, D. Kovalev, J. Diener, F. Koch, S. Takeoka and S. Hayashi: J. Appl. Phys. 88 (2000) 5772[AIP Scitation].
  18. T. Matsumoto, Y. Masumoto, T. Nakagawa, M. Hashimoto, K. Ueno and N. Koshida: Jpn. J. Appl. Phys. 36 (1997) L1089[JSAP].
  19. B. Gelloz, A. Kojima and N. Koshida: Appl. Phys. Lett. 87 (2005) 031107[AIP Scitation].
  20. B. Gelloz and N. Koshida: J. Appl. Phys. 98 (2005) 123509[AIP Scitation].
  21. M. Fujii, A. Mimura, S. Hayashi, Y. Yamamoto and K. Murakami: Phys. Rev. Lett. 89 (2002) 206805[APS].
  22. M. Fujii, A. Mimura, S. Hayashi and K. Yamamoto: Appl. Phys. Lett. 75 (1999) 184[AIP Scitation].
  23. M. Fujii, A. Mimura, S. Hayashi, K. Yamamoto, C. Urakawa and H. Ohta: J. Appl. Phys. 87 (2000) 1855[AIP Scitation].
  24. K. Toshikiyo, M. Tokunaga, S. Takeoka, M. Fujii, S. Hayashi and K. Moriwaki: J. Appl. Phys. 90 (2001) 5147[AIP Scitation].
  25. K. Matsumoto, K. Imakita, M. Fujii and S. Hayashi: Jpn. J. Appl. Phys. 44 (2005) L1547[JSAP].
  26. A. Irrera, D. Pacifici, M. Miritello, G. Franzó, F. Priolo, F. Iacona, D. Sanfilippo, G. Di Stefano and P. G. Fallica: Appl. Phys. Lett. 81 (2002) 1866[AIP Scitation].
  27. Y. Yamada, N. Suzuki, T. Makino and T. Yoshida: J. Vac. Sci. Technol. A 18 (2000) 83[AIP Scitation].
  28. Y. Kanzawa, M. Fujii, S. Hayashi and K. Yamamoto: Solid State Commun. 100 (1996) 227[CrossRef].
  29. M. Fujii, S. Hayashi and K. Yamamoto: J. Appl. Phys. 83 (1998) 7953[AIP Scitation].

|TOP|  |Previous Article| |Next Article|  |Table of Contents| |JJAP Home|
Copyright © 2013 The Japan Society of Applied Physics
Contact Information