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Jpn. J. Appl. Phys. 50 (2011) 01AJ03 (4 pages)  |Previous Article| |Next Article|  |Table of Contents|
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Visible Light-Induced Catalytic Oxidation Using Zeolite Encapsulating Two Distinct Metal Complexes

Tomohiko Inomata, Yoshimasa Nagai, Nayumi Ohata, Yasuhiro Funahashi, Tomohiro Ozawa, and Hideki Masuda

Department of Material Science and Engineering, Graduate School of Engineering, Nagoya Institute of Technology, Nagoya 466-8555, Japan

(Received April 30, 2010; accepted August 26, 2010; published online January 20, 2011)

Y-type zeolite encapsulating two distinct metal complexes has been synthesized. This zeolite contains Ru(bpy)3 (bpy = 2,2'-bipyridine) and Mn(saloph) [saloph = N,N'-bis(salicylidene)-o-phenylenediamine] as photoinducing and oxidative catalytic sites, respectively. The zeolite showed the quenching of the emission, resulting in the effective electron/energy transfer from the RuII center to the MnII center in it. The oxidation reaction of dimethyl sulfide with the zeolite has been accelerated by photoirradiation. This phenomenon indicates that the electron/energy transfer from Ru(bpy)3 units affects the oxidation reaction on Mn(saloph) units.

URL: http://jjap.jsap.jp/link?JJAP/50/01AJ03/
DOI: 10.1143/JJAP.50.01AJ03
PACS: 82.75.Qt, 82.75.Fq, 78.40.Me


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